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Methods of increasing the performance of radionuclide generators used in nuclear medicine daughter nuclide build up optimisation, elution purification concentration integration, and effective control of radionuclidic

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Nội dung chi tiết: Methods of increasing the performance of radionuclide generators used in nuclear medicine daughter nuclide build up optimisation, elution purification concentration integration, and effective control of radionuclidic

Methods of increasing the performance of radionuclide generators used in nuclear medicine daughter nuclide build up optimisation, elution purification concentration integration, and effective control of radionuclidic

Molecules 2014. 19. 7714-7756: doi: 10.3390 molecules 19067714OPEN ACCESSmoleculesISSN 1420-3049 www.mdpi com journalmolecules ArticleMethods of Incre

Methods of increasing the performance of radionuclide generators used in nuclear medicine daughter nuclide build up optimisation, elution purification concentration integration, and effective control of radionuclidic easing the Performance of Radionuclide Generators Used in Nuclear Medicine: Daughter Nuclide Build-Up Optimisation, Elution-Purification-Concentration

Integration, and Effective Control of Radionuclidic PurityX an So Le 1’2'*, Zoe Phuc-llien Do Ả Minh Khoi Le 2, Vicki Le 2 and Natalie Nha-Truc Le 21 Methods of increasing the performance of radionuclide generators used in nuclear medicine daughter nuclide build up optimisation, elution purification concentration integration, and effective control of radionuclidic

Cyclophaim Lid.. Sydney 223'1. NSW. Australia■ Medical Isotope Techniques (MF.DTSOTFC), I4( I) Dwyer Street. Gymea 2227, NSW. Australia: E-Mails: soh

Methods of increasing the performance of radionuclide generators used in nuclear medicine daughter nuclide build up optimisation, elution purification concentration integration, and effective control of radionuclidic

ien tvk@yahoo.com (7..P.-H.D ); minh.kh.le@gmail.com (M.K.L.); vi_3001@holurail.com (V.L.): nalalie.nl.dubs@gmail.com (N.N.-l.L.)* Author to whom corr

Molecules 2014. 19. 7714-7756: doi: 10.3390 molecules 19067714OPEN ACCESSmoleculesISSN 1420-3049 www.mdpi com journalmolecules ArticleMethods of Incre

Methods of increasing the performance of radionuclide generators used in nuclear medicine daughter nuclide build up optimisation, elution purification concentration integration, and effective control of radionuclidic pted: 5 June 2014 /Published: 10 June 2014Abstract: Methods of increasing the performance of radionuclide generators used in nuclear medicine radiothe

rapy and SPEC 1 PL 1 imaging were developed and detailed for "Mo/^'Tc and ’’Ge /6sGa radionuclide generators as the cases. Optimisation methods of the Methods of increasing the performance of radionuclide generators used in nuclear medicine daughter nuclide build up optimisation, elution purification concentration integration, and effective control of radionuclidic

daughter nuclide build-up versus stand-by lime and or specific activity using mean progress functions were dev eloped for increasing the performance

Methods of increasing the performance of radionuclide generators used in nuclear medicine daughter nuclide build up optimisation, elution purification concentration integration, and effective control of radionuclidic

of radionuclide generators. As a result of this optimisation, rhe separation of rhe daughter nuclide from its parent one should be performed al a defi

Molecules 2014. 19. 7714-7756: doi: 10.3390 molecules 19067714OPEN ACCESSmoleculesISSN 1420-3049 www.mdpi com journalmolecules ArticleMethods of Incre

Methods of increasing the performance of radionuclide generators used in nuclear medicine daughter nuclide build up optimisation, elution purification concentration integration, and effective control of radionuclidic r nuclide yield is maintained to a reasonably high extent. A new characteristic parameter of the formation-decay kinetics of parent daughter nuclide s

ystem was found and effectively used in the practice of the generator production and utilisation. A method of “early elution schedule” was also develo Methods of increasing the performance of radionuclide generators used in nuclear medicine daughter nuclide build up optimisation, elution purification concentration integration, and effective control of radionuclidic

ped for increasing the daughter nuclide production yield and specific radioactivity, thus saving the cost of the generator and improv mg the quality o

Methods of increasing the performance of radionuclide generators used in nuclear medicine daughter nuclide build up optimisation, elution purification concentration integration, and effective control of radionuclidic

f the daughter radionuclide solution. These newly developed optimisation methods 111 combination with an integrated elution-pui ification-concentratio

Molecules 2014. 19. 7714-7756: doi: 10.3390 molecules 19067714OPEN ACCESSmoleculesISSN 1420-3049 www.mdpi com journalmolecules ArticleMethods of Incre

Methods of increasing the performance of radionuclide generators used in nuclear medicine daughter nuclide build up optimisation, elution purification concentration integration, and effective control of radionuclidic improvement of purposely suitable quality and specific activity of the produced daughter radionuclides All these features benefit the economic use ofM

olecules 2014. /97715the generator, the improved quality of labelling scan, and the lowered cost of nuclear medicine procedure. Besides, a new method Methods of increasing the performance of radionuclide generators used in nuclear medicine daughter nuclide build up optimisation, elution purification concentration integration, and effective control of radionuclidic

of quality control piotocol set-up for post-delivery test of radionuclidic purity has been developed based on the relationship between gamma ray spect

Methods of increasing the performance of radionuclide generators used in nuclear medicine daughter nuclide build up optimisation, elution purification concentration integration, and effective control of radionuclidic

rometric detection limit, required limit of impure radionuclide activity and its measurement certainty with respect to optimising decay measurement ti

Molecules 2014. 19. 7714-7756: doi: 10.3390 molecules 19067714OPEN ACCESSmoleculesISSN 1420-3049 www.mdpi com journalmolecules ArticleMethods of Incre

Methods of increasing the performance of radionuclide generators used in nuclear medicine daughter nuclide build up optimisation, elution purification concentration integration, and effective control of radionuclidic d avoids wasting the useful amount of valuable purified concentrated daughter nuclide product. This process is important for the spectrometric measure

ment of very low activity of impure radionuclide contamination in the radioisotope products of much higher activity used ill medical imaging and targe Methods of increasing the performance of radionuclide generators used in nuclear medicine daughter nuclide build up optimisation, elution purification concentration integration, and effective control of radionuclidic

ted radiotherapy.Keywords: radionuclide generator" radioisotope concentrator; mean progress function; optimal build-up time: effective specific activi

Methods of increasing the performance of radionuclide generators used in nuclear medicine daughter nuclide build up optimisation, elution purification concentration integration, and effective control of radionuclidic

ty; radionuclidic purity; nuclear medicine: radiopharmaceutical: ‘WmTc; 6SGa1. IntroductionToday most radionuclide generators are used for nuclear med

Molecules 2014. 19. 7714-7756: doi: 10.3390 molecules 19067714OPEN ACCESSmoleculesISSN 1420-3049 www.mdpi com journalmolecules ArticleMethods of Incre

Methods of increasing the performance of radionuclide generators used in nuclear medicine daughter nuclide build up optimisation, elution purification concentration integration, and effective control of radionuclidic Sr/'^Rb, 6*Gc?sGa. KZiA’u, 18*W/188Rc, *»Sr/*>Y, and l<*Dy/lwllo among which the "Mo/^Tc generator is used most effectively. Other generator systems a

re used to some extent or are under development. More than 80% of diagnostic imaging procedures of nuclear medicine based on ?'"Tc-radiophaimaceutical Methods of increasing the performance of radionuclide generators used in nuclear medicine daughter nuclide build up optimisation, elution purification concentration integration, and effective control of radionuclidic

s are performed world-wide every year, rhe short-lived gamma or positron emitting radioisotopes produced from radionuclide generators are effectively

Methods of increasing the performance of radionuclide generators used in nuclear medicine daughter nuclide build up optimisation, elution purification concentration integration, and effective control of radionuclidic

used in diagnostic nuclear medicine and in biomedical research, while the generator-produced long-lived beta- and alpha-emitting radioisotopes are use

Molecules 2014. 19. 7714-7756: doi: 10.3390 molecules 19067714OPEN ACCESSmoleculesISSN 1420-3049 www.mdpi com journalmolecules ArticleMethods of Incre

Methods of increasing the performance of radionuclide generators used in nuclear medicine daughter nuclide build up optimisation, elution purification concentration integration, and effective control of radionuclidic sGa and ’’Rb in positron emission tomography (PEI) for diagnostic imaging. Expansion of the use of radionuclides produced hour radionuclide generators

IS always desirable, subsequently benefiting superiority of the SPEC! and PFT-based molecular imaging technique Usually, a radionuclide generator, or Methods of increasing the performance of radionuclide generators used in nuclear medicine daughter nuclide build up optimisation, elution purification concentration integration, and effective control of radionuclidic

colloquially a “radioisotope cow” IS a device used to extract the short-lived daughter nuclide generated fiom the radioactive decay of long-lived par

Methods of increasing the performance of radionuclide generators used in nuclear medicine daughter nuclide build up optimisation, elution purification concentration integration, and effective control of radionuclidic

ent nuclide. As such. It can be easily transported over long distances to radiopharmacies where its decay product daughter radionuclide is extracted f

Molecules 2014. 19. 7714-7756: doi: 10.3390 molecules 19067714OPEN ACCESSmoleculesISSN 1420-3049 www.mdpi com journalmolecules ArticleMethods of Incre

Methods of increasing the performance of radionuclide generators used in nuclear medicine daughter nuclide build up optimisation, elution purification concentration integration, and effective control of radionuclidic r, the acceptability of a radionuclide generator to be used HI nuclear diagnostic therapeutic procedures and the quality of SPECT imaging diagnosis an

d or endo-radiotherapy are controlled by the generator design and Its operation management “daughter nuclide milking” schedule. The efficacy of a radi Methods of increasing the performance of radionuclide generators used in nuclear medicine daughter nuclide build up optimisation, elution purification concentration integration, and effective control of radionuclidic

onuclide generator used in nuclear medicine depends on the concentration and specific radioactivity (SX) of the daughter nuclide in the solution produ

Methods of increasing the performance of radionuclide generators used in nuclear medicine daughter nuclide build up optimisation, elution purification concentration integration, and effective control of radionuclidic

ced from the generator, because the volume and the mass of bio-medically active radiolabelled agents used 111 oneMolecules 2014.197716given injection

Molecules 2014. 19. 7714-7756: doi: 10.3390 molecules 19067714OPEN ACCESSmoleculesISSN 1420-3049 www.mdpi com journalmolecules ArticleMethods of Incre

Methods of increasing the performance of radionuclide generators used in nuclear medicine daughter nuclide build up optimisation, elution purification concentration integration, and effective control of radionuclidic ody. Daughter nuclide concentration is determined by the radioactivity yield of each “milking’Vehition of the generator and the final volume of the da

ughter nuclide solution. Illis solution volume is fixed and defined by the generator design which is dictated by a given radiochemical processing proc Methods of increasing the performance of radionuclide generators used in nuclear medicine daughter nuclide build up optimisation, elution purification concentration integration, and effective control of radionuclidic

ess. However, the specific radioactivity of (S.-Í) of the daughter nuclide IS affected by the "milking" schedule only.Additionally, the cost-effective

Methods of increasing the performance of radionuclide generators used in nuclear medicine daughter nuclide build up optimisation, elution purification concentration integration, and effective control of radionuclidic

utilisation of the generator is controlled by the daughter nuclide yield obtained fol the whole lifetime of a given generator, which is the sum of yi

Molecules 2014. 19. 7714-7756: doi: 10.3390 molecules 19067714OPEN ACCESSmoleculesISSN 1420-3049 www.mdpi com journalmolecules ArticleMethods of Incre

Methods of increasing the performance of radionuclide generators used in nuclear medicine daughter nuclide build up optimisation, elution purification concentration integration, and effective control of radionuclidic enerator. Ill conclusion, for an established design of generator system, the build-up lime schedule of the daughter nuclide for the generator operatio

n management will determine not only the concentration and specific radioactivity of the daughter nuclide solution obtained from the generator but als Methods of increasing the performance of radionuclide generators used in nuclear medicine daughter nuclide build up optimisation, elution purification concentration integration, and effective control of radionuclidic

o the cost-effective utilisation of the generator system. Hills the effective utilisation of the generator is experienced as a result of proper “milki

Methods of increasing the performance of radionuclide generators used in nuclear medicine daughter nuclide build up optimisation, elution purification concentration integration, and effective control of radionuclidic

ng" management based on the optimal schedule of the daughter nuclide build-up time. Similarly, the optimisation in the daughter nuclide decay lime sch

Molecules 2014. 19. 7714-7756: doi: 10.3390 molecules 19067714OPEN ACCESSmoleculesISSN 1420-3049 www.mdpi com journalmolecules ArticleMethods of Incre

Methods of increasing the performance of radionuclide generators used in nuclear medicine daughter nuclide build up optimisation, elution purification concentration integration, and effective control of radionuclidic erefore the report on this issue is also included in this article.With lire success in the development of the integrated elulioii-puiificalioii-concen

lialion systems (RADIGIS-Radioisotopc Generator Integrated System) and the radioisotope concentrator device UT.TRAT.UTF/ to achieve a small volume (- Methods of increasing the performance of radionuclide generators used in nuclear medicine daughter nuclide build up optimisation, elution purification concentration integration, and effective control of radionuclidic

1.0 mT.) of the product solution of daughter nuclide obtained fiom the variable design of the generator systems as reported in our previous papers fl-

Methods of increasing the performance of radionuclide generators used in nuclear medicine daughter nuclide build up optimisation, elution purification concentration integration, and effective control of radionuclidic

101, the optimisation methods of radionuclide generator operation management as mentioned above w ill in turn become rhe most important subject to be

Molecules 2014. 19. 7714-7756: doi: 10.3390 molecules 19067714OPEN ACCESSmoleculesISSN 1420-3049 www.mdpi com journalmolecules ArticleMethods of Incre

Methods of increasing the performance of radionuclide generators used in nuclear medicine daughter nuclide build up optimisation, elution purification concentration integration, and effective control of radionuclidic nd-by lime of the generator for each “milking”) for the generator operation have been available ill the literature until now. Our present work is focu

sed on providing the optimisation methods first time developed for the radionuclide generator operation management lo increase the effectiveness of th Methods of increasing the performance of radionuclide generators used in nuclear medicine daughter nuclide build up optimisation, elution purification concentration integration, and effective control of radionuclidic

e radionuclide generator utilisation.2. Theoretical Approach and Method Development2.1. Daughter Nuclide Build-Up Optimisation for Improvement of Prod

Methods of increasing the performance of radionuclide generators used in nuclear medicine daughter nuclide build up optimisation, elution purification concentration integration, and effective control of radionuclidic

uction Yield and Specific Rad ioacti 1 7Ạ •General consideration: For the reason of ensuring a convenient and effective radiochemical separation, the

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