Catalytic intramolecular carbene transfer reactions into σ and π bonds
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Catalytic intramolecular carbene transfer reactions into σ and π bonds
Catalytic Intramolecular Carbene Transfer Reactions intoƠ and 71 BondsMarch, 2020Doctor of Philosophy (Engineering)PHAN THI THANH NGA77?jfToyohashi Un Catalytic intramolecular carbene transfer reactions into σ and π bonds niversity of TechnologyACKNOWLEDGEMENTSFirst and foremost. I would like to express my deep thanks to my supervisor. Professor Dr. Seiji Ivvasa, for everything he did for me during my study within four years. Actually, there is no words can express my deep sense of gratitude towards him. I would like Catalytic intramolecular carbene transfer reactions into σ and π bonds to thanks him for his endless support, encouragement, advices and patience throughout my PhD work.I would like to express Prof. Dr. Kazutaka ShibatomCatalytic intramolecular carbene transfer reactions into σ and π bonds
i for his investing time and providing interesting and valuable feedback throughout my research period.And I would like to thank to my doctoral commitCatalytic Intramolecular Carbene Transfer Reactions intoƠ and 71 BondsMarch, 2020Doctor of Philosophy (Engineering)PHAN THI THANH NGA77?jfToyohashi Un Catalytic intramolecular carbene transfer reactions into σ and π bonds th the X-ray measurements. I am very grateful to Mr. Masaya Tone. Mr. Hayato Inoue. Ms. Huong for their cooperation, suggestion, and valuable discussion throughout my research period.I also would like to acknowledge all the labmates whom I had the pleasure of working with: Dr. Soda, Dr. Hamada, Dr. Catalytic intramolecular carbene transfer reactions into σ and π bonds Kotozaki, Dr. Nakagawa, Dr. Chi, Ms. Doan, Mr. Angus. Mr. Liang. Mr. Fujii. Mr. Fukuda. Ms. Nansalmaa. Ms. Matozaki. Mr. Ogura. Mr. Yamaguchi. Ms. LinCatalytic intramolecular carbene transfer reactions into σ and π bonds
hda. Ms. Zolzaya and all other research scholars of tile department who have been very friendly and helped me in various ways.I acknowledge all the stCatalytic Intramolecular Carbene Transfer Reactions intoƠ and 71 BondsMarch, 2020Doctor of Philosophy (Engineering)PHAN THI THANH NGA77?jfToyohashi Un Catalytic intramolecular carbene transfer reactions into σ and π bonds aduation steps.I would like to thank all the friends that I have met in Toyohashi: Mona. Hang. Hue. B«ão. Trinh, Hường, Khôn. Hoài. I really cherish the great time we spent together: the dinner parties, summer barbecues, autumn red leaves, skiing and Tet.With my appreciation and respect, this work w Catalytic intramolecular carbene transfer reactions into σ and π bonds ould not have been possible without the financial support of the Hitachi Global Foundation, they gave me the chance to study in Japan under their finaCatalytic intramolecular carbene transfer reactions into σ and π bonds
ncial support to my work.I want to thank all the staffs of Faculty of Chemical Engineering. HCMC University of Technology for their supports in the fuCatalytic Intramolecular Carbene Transfer Reactions intoƠ and 71 BondsMarch, 2020Doctor of Philosophy (Engineering)PHAN THI THANH NGA77?jfToyohashi Un Catalytic intramolecular carbene transfer reactions into σ and π bonds pport and encouragement.My deepest gratitude is reserved for my family, for having filled my life with every’ joy. helping me to get through so many gloomy days and lighting up every last comer. For my parents, my brother Án who have always been there for me. Needless to say. they have helped immeas Catalytic intramolecular carbene transfer reactions into σ and π bonds urably to get me to tins point in my life.Thank you very much!PHAN THI THANH NGADepartment of Applied Chemistry and Life ScienceToyohashi University oCatalytic intramolecular carbene transfer reactions into σ and π bonds
f Technology. 1-1 Tempaku-cho.Toyohashi. Aichi 441-8580 (Japan)E-mail: phanthanhngafr hcmut.edu.vniiABSTRACTKeywords: asymmetric synthesis, cyclop!opaCatalytic Intramolecular Carbene Transfer Reactions intoƠ and 71 BondsMarch, 2020Doctor of Philosophy (Engineering)PHAN THI THANH NGA77?jfToyohashi Un Catalytic intramolecular carbene transfer reactions into σ and π bonds orresponding metal-carbene complex and catalytically inserts into 0 and 7t bonds of the organic compound. Even though there are many reports on the carbene transfer process to develop a new approach for the synthesis of medicine and other bioactive compounds, the regio-, stereo- and chemoselective a Catalytic intramolecular carbene transfer reactions into σ and π bonds pproaches are still limited and remained as the mam subject in the field of synthetic organic chemistry. For this background. I developed an efficientCatalytic intramolecular carbene transfer reactions into σ and π bonds
catalytic intramolecular carbene transfer reactions by using originally developed nitheniiun catalyst into Ơ and ỈĨ bonds and successfully applied foCatalytic Intramolecular Carbene Transfer Reactions intoƠ and 71 BondsMarch, 2020Doctor of Philosophy (Engineering)PHAN THI THANH NGA77?jfToyohashi Un Catalytic intramolecular carbene transfer reactions into σ and π bonds hner reactionAlthough the ruthenium complex is a newcomer in the field of catalytic carbene transfer reaction, it has emerged as a useful transition metal for the carbenoid chemistry' of diazo compounds, besides copper and rhodium. And recently, we have developed a Ru(II)-Pheox complex, which IS eff Catalytic intramolecular carbene transfer reactions into σ and π bonds icient for carbene transfer reactions, in particular, asymmetric cyclopropanation. N-H insertion. C-H insertion and S1-H insertion reactions.ThereforeCatalytic intramolecular carbene transfer reactions into σ and π bonds
, driven by my interests in the catalytic asymmetric carbene transfer reaction and the efficiency displayed by the Ru(II)-Pheox catalyst. I started toCatalytic Intramolecular Carbene Transfer Reactions intoƠ and 71 BondsMarch, 2020Doctor of Philosophy (Engineering)PHAN THI THANH NGA77?jfToyohashi Un Catalytic intramolecular carbene transfer reactions into σ and π bonds tant to be applied in pharmaceutical and medicinal fields.In my thesis. Chapter 1 describes the importance of carbene transfer reactions. And a short review of the metal carbene intermediates in C-H insertion, asymmetric cycloplopanations. and Buchner reaction have been also illustrated in this chap Catalytic intramolecular carbene transfer reactions into σ and π bonds ter hl addition, the application of metal carbene complexes 111 the synthesis of biologically-active or natural product-like compounds is also mentionCatalytic intramolecular carbene transfer reactions into σ and π bonds
ed.Chapter 2 is for the synthesis of oxmdoles. The oxindole ring IS prevalent as an important scaffold found 111 munerous natural products and pharmacCatalytic Intramolecular Carbene Transfer Reactions intoƠ and 71 BondsMarch, 2020Doctor of Philosophy (Engineering)PHAN THI THANH NGA77?jfToyohashi Un Catalytic intramolecular carbene transfer reactions into σ and π bonds inal chemists to synthesize novel oxindole derivatives. I report Ru(II)-PheoxiiiCatalytic Intramolecular Carbene Transfer Reactions intoƠ and 71 BondsMarch, 2020Doctor of Philosophy (Engineering)PHAN THI THANH NGA77?jfToyohashi UnGọi ngay
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